2,2,2-Trifluoro-N-(isoquinolin-5-ylmethyl)acetamide

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2,2,2-Trifluoro-N-(isoquinolin-5-ylmeth­yl)acetamide

The mol-ecular structure of the title compound at 123 K, C(12)H(9)F(3)N(2)O, presents a rotationally disordered CF(3) group. Hydrogen bonds between the amide NH group and the N atom of the isoquinoline form a chain in the b-axis direction. The packed structure forms alternate layers of isoquinoline and amide groups parallel to the ab plane.

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N-(4-Chloro­phen­yl)-1,1,1-trifluoro-N-(trifluoro­methyl­sulfon­yl)methane­sulfonamide

The title mol-ecule, also called 4-chloro-N,N-bis-(trifluoro-methane-sulfon-yl)aniline, C(8)H(4)ClF(6)NO(4)S(2), has non-crystallographic twofold symmetry with the pseudo-axis aligned along the Cl-C⋯C-N backbone of the mol-ecule: the SO(2)CF(3) residues lie to either side of the benzene ring. In the crystal, the presence of C-H⋯O contacts lead to the formation of a sequence of 12-membered {⋯HC(...

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7-Chloro-1,2-dihydro­furo[2,3-c]isoquinolin-5-amine

In the title compound, C(11)H(9)ClN(2)O, the fused-ring system is essentially planar, with a maximum deviation of 0.0323 (16) Å. In the crystal, mol-ecules are connected by N-H⋯O hydrogen bonds forming a zigzag chain along the c axis. Mol-ecules are further stacked along the a axis through weak π-π inter-actions, the shortest distance between ring centroids being 3.6476 (8) Å.

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N-[3-(2-Methyl­phen­yl)isoquinolin-1-yl]formamide

The title compound, C(17)H(14)N(2)O, crystallizes as a cis formamide isomer. The isoquinoline and benzene fragments are nearly perpendicular [dihedral angle = 81.79 (18)°], whereas the formamide group is virtually coplanar with the isoquinoline unit [dihedral angle = 1.66 (15)°]. Inter-molecular N-H⋯O hydrogen bonds link mol-ecules into a centrosymmetric dimer.

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A simple access to N-(un)substituted isoquinolin-1(2H)-ones: unusual formation of regioisomeric isoquinolin-1(4H)-ones.

A ligand/additive/Pd-free Cu-mediated coupling/cyclization strategy afforded the first practical, one-pot and general approach towards synthesis of N-(un)substituted isoquinolin-1(2H)-ones. Both the catalyst and the solvent used are recyclable. The use of the Cu reagent in excess led to the unusual formation of regioisomeric and uncommon isoquinolin-1(4H)-ones.

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ژورنال

عنوان ژورنال: Acta Crystallographica Section E Structure Reports Online

سال: 2009

ISSN: 1600-5368

DOI: 10.1107/s1600536809052994